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In the mid-1830s, the United States learned that it was the beneficiary of a strange and unprecedented bequest. An Englishman named James Smithson, who had never set foot in the U.S., had left all his fortune to found in Washington "an establishment for the increase and diffusion of knowledge among men." He left no further instructions, and the questions surrounding the extraordinary bequest sparked a rancorous decade-long debate in Congress. Since its founding in 1846, the Smithsonian Institution has grown into the largest museum and research complex in the world. Known as "the Nation's Attic," it is the keeper of many of America's most treasured cultural icons-the Star-Spangled Banner, the Spirit of St. Louis, Lincoln's top hat, and Dorothy's ruby slippers. At its heart, however, has always been the mystery of its enigmatic benefactor. Drawing on unpublished letters and diaries from archives across Europe and the United States-including the entirety of the Smithsonian's...